You might want to provide more details on what you are specifically
trying to accomplish - are you looking to automate this process to
be run regularly, or is it just a one-time task? Are there a lot of
documents to be copied?
If it is just a one-time thing, I'd say the easiest way to do this
is not through code, but to go to your document library, switch to
Explorer View, right-click and copy the files from that document
library you want to bring into the new one, and paste them into the
new one (also using Explorer View). Then again you might have a lot
of documents in the document library and might not want to rummage
through the entire library, but I don't know for sure.